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<title>Ultrafast Metal‐Free Microsupercapacitor Arrays Directly Store Instantaneous High‐Voltage Electricity from Mechanical Energy Harvesters</title>
<creator>Chen, Shiqian</creator>
<creator>Li, Zheng</creator>
<creator>Huang, Po‐Han</creator>
<creator>Ruiz Fernández, Virginia</creator>
<creator>Su, Yingchun</creator>
<creator>Fu, Yujie</creator>
<creator>Alesanco, Yolanda</creator>
<creator>Malm, B. Gunnar</creator>
<creator>Niklaus, Frank</creator>
<creator>Li, Jiantong</creator>
<subject>Droplet-based electrcity generators</subject>
<subject>Full printing</subject>
<subject>Microsupercapacitor arrays</subject>
<subject>On-paper electronics</subject>
<subject>PEDOT:PSS</subject>
<description>Harvesting renewable mechanical energy is envisioned as a promising and sustainable way for power generation. Many recent mechanical energy harvesters are able to produce instantaneous (pulsed) electricity with a high peak voltage of over 100 V. However, directly storing such irregular high-voltage pulse electricity remains a great challenge. The use of extra power management components can boost storage efficiency but increase system complexity. Here utilizing the conducting polymer PEDOT:PSS, high-rate metal-free micro-supercapacitor (MSC) arrays are successfully fabricated for direct high-efficiency storage of high-voltage pulse electricity. Within an area of 2.4 × 3.4 cm2 on various paper substrates, large-scale MSC arrays (comprising up to 100 cells) can be printed to deliver a working voltage window of 160 V at an ultrahigh scan rate up to 30 V s−1. The ultrahigh rate capability enables the MSC arrays to quickly capture and efficiently store the high-voltage (≈150 V) pulse electricity produced by a droplet-based electricity generator at a high efficiency of 62%, significantly higher than that (&lt;2%) of the batteries or capacitors demonstrated in the literature. Moreover, the compact and metal-free features make these MSC arrays excellent candidates for sustainable high-performance energy storage in self-charging power systems.</description>
<date>2025-03-10</date>
<date>2025-03-10</date>
<date>2024-03</date>
<type>info:eu-repo/semantics/article</type>
<identifier>2198-3844</identifier>
<identifier>http://hdl.handle.net/10259/10299</identifier>
<identifier>10.1002/advs.202400697</identifier>
<identifier>2198-3844</identifier>
<language>eng</language>
<relation>Advanced Science. 2024, V. 11, n. 22, p. 2400697</relation>
<relation>https://doi.org/10.1002/advs.202400697</relation>
<rights>http://creativecommons.org/licenses/by/4.0/</rights>
<rights>info:eu-repo/semantics/openAccess</rights>
<rights>Atribución 4.0 Internacional</rights>
<publisher>Wiley</publisher>
</thesis></metadata></record></GetRecord></OAI-PMH>