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<mods:namePart>Li, Zheng</mods:namePart>
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<mods:namePart>Li, Yuanyuan</mods:namePart>
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<mods:namePart>Zhuang, Xiaodong</mods:namePart>
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<mods:namePart>Weissenrieder, Jonas</mods:namePart>
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<mods:namePart>Cheng, Shi</mods:namePart>
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<mods:namePart>Li, Jiantong</mods:namePart>
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<mods:dateAccessioned encoding="iso8601">2025-03-11T07:54:18Z</mods:dateAccessioned>
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<mods:dateIssued encoding="iso8601">2021-10</mods:dateIssued>
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<mods:identifier type="issn">1616-301X</mods:identifier>
<mods:identifier type="uri">http://hdl.handle.net/10259/10300</mods:identifier>
<mods:identifier type="doi">10.1002/adfm.202108773</mods:identifier>
<mods:identifier type="essn">1616-3028</mods:identifier>
<mods:abstract>On-paper microsupercapacitors (MSCs) are a key energy storage component for disposable electronics that are anticipated to essentially address the increasing global concern of electronic waste. However, nearly none of the present on-paper MSCs combine eco-friendliness with high electrochemical performance (especially the rate capacity). In this work, highly reliable conductive inks based on the ternary composite of poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PEDOT:PSS), graphene quantum dots and graphene are developed for scalable inkjet printing of compact (footprint area ≈ 20 mm2) disposable MSCs on commercial paper substrates. Without any post treatment, the printed patterns attain a sheet resistance as low as 4 Ω ▫−1. The metal-free all-solid-state MSCs exhibit a maximum areal capacitance > 2 mF cm−2 at a high scan rate of 1000 mV s−1, long cycle life (>95% capacitance retention after 10 000 cycles), excellent flexibility, and long service time. Remarkably, the “totally metal-free” MSC arrays are fully inkjet printed on paper substrates and also exhibit high rate performance. The life cycle assessment indicates that these printed devices have much lower eco-toxicity and global warming potential than other on-paper MSCs.</mods:abstract>
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<mods:accessCondition type="useAndReproduction">Attribution-NonCommercial-NoDerivatives 4.0 Internacional</mods:accessCondition>
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<mods:topic>Disposable electronics</mods:topic>
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<mods:subject>
<mods:topic>Electrochemically exfoliated graphene</mods:topic>
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<mods:topic>Graphene quantum dots</mods:topic>
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<mods:topic>Inkjet printing</mods:topic>
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<mods:topic>On-paper microsupercapacitors</mods:topic>
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<mods:subject>
<mods:topic>PEDOT:PSS</mods:topic>
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<mods:titleInfo>
<mods:title>Inkjet Printed Disposable High‐Rate On‐Paper Microsupercapacitors</mods:title>
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